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Impact ionization processes in a photodriven Mott insulator: Influence of phononic dissipation

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Abstract

We study a model for photovoltaic energy collection consisting of a Mott-insulating layer in presence of acoustic phonons, coupled to two wide-band fermion leads at different chemical potentials and driven into a nonequilibrium steady state by a periodic electric field. We treat electron correlations with nonequilibrium dynamical mean-field theory using the so-called auxiliary master-equation approach as impurity solver and include dissipation by acoustic phonons via the Migdal approximation. For a small hybridization to the leads, we obtain a peak in the photocurrent as a function of the driving frequency which can be associated with impact ionization processes. For larger hybridizations the shallow peak suggests a suppression of impact ionization with respect to direct photovoltaic excitations. Acoustic phonons slightly enhance the photocurrent for small driving frequencies and suppress it at frequencies around the main peak at all considered hybridization strengths.
Original languageEnglish
Article number195140
JournalPhysical Review B
Volume106
Issue number19
DOIs
Publication statusPublished - 15 Nov 2022

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 7 - Affordable and Clean Energy
    SDG 7 Affordable and Clean Energy

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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